So you can confirm the theory, we customized and you will waiting a great multicomponent copolymer by significant cross-linked copolymerization away from gas acid and you can several luminophores (Fig. 1c). At the same time, the formation of a mix-connected polymer circle can get then enhance the rigidity out of polymer matrix to possess generating a lot of time-resided phosphorescence emission lower than ambient requirements. B Stabilized phosphorescence spectra away from monomer MDP and MND inside two-methyltetrahydrofuran (1 × 10−5 M) from the 77 K (top), in addition to polymer PDA and you can PNA during the room-temperature (RT) (bottom) thrilled in the 280 and you will 360 nm. C Polymer movie excitation–phosphorescence mapping out of PDA (top) and you can PNA (bottom) on the space-heat. Age Sheer alter orbitals on the lower triplet transitions away from MDP and you will MND to the gaseous condition.

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It must be pointed out that the received display an enormous difference in fluorescence and you can phosphorescence emission, which happen to be perfect for steer clear of the listing disturbance and you might fluorescence come across-quenching. Including, the essential difference between the brand new fluorescence emission wavelength and you could possibly get phosphorescence emission wavelength out of and you may product is to the 70 and 130 nm, respectively (Figs. S20 and you can S23). To help you clarify the formation of triplet says for long-stayed emission, i analyzed the brand new character away from triplet generation by the transient assimilation (TA) studies for the PSSNa polymer motion picture (Supplementary Fig. 34).

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